I use Google Music (Play Music?) and plug my S3 into my computer with iTunes and my music. It all transferred without a problem.
What I post is my 2 cents and nothing more. Please don't read anything into my post that's not there. If you disagree, that's OK. Can't we all just get along?
Doubletwist lets ypu sync iTunes with Android phones.
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The iSyncr app from the Google play store does it really easily. Install it on your phone & computer & follow the very easy instructions. You can use Samsung Kies as well but I personally have not used it.
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